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周祎副教授、宋波教授与李永舫院士合作在J. Mater. Chem. A上发表研究论文
 Room-temperature mixed-solvent-vapor annealing for high performance perovskite solar cells

Hao Yu,a  Xiaodong Liu,a  Yijun Xia,a  Qingqing Dong,a  Kaicheng Zhang,a  Zhaowei Wang,a   Yi Zhou,*a   Bo Song*a and   Yongfang Li*ab

 

a Laboratory of Advanced Optoelectronic Materials, College of Chemistry, Chemical Engineering and Materials Science, Soochow University, Suzhou, China

b Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing, China

 

J. Mater. Chem. A, 2016,4, 321-326

 

In this paper, we introduce a room-temperature mixed-solvent-vapor annealing (rtMSVA) method to fabricate high performance perovskite solar cells (pero-SCs) based on MAPbI3−xClx without the need for thermal annealing (TA). An ultra-smooth perovskite thin-film with high crystallinity was obtained by the DMF/CB mixed-solvent (1:20, v/v) vapor annealing at room-temperature without TA and the power conversion efficiency (PCE) of the pero-SCs reached 16.4%. More importantly, the reproducibility of the PCEs is quite good among 40 different devices. Furthermore, large active area pero-SCs were fabricated with the rtMSVA method. The PCEs of the pero-SCs based on ITO and flexible PET/Ag mesh electrodes with an active area of 1.21 cm2 reached 11.01% and 7.5%, respectively. We anticipate that rtMSVA would very possibly become a promising crystallization method for the fabrication of large area pero-SCs in the near future.

                           

链接://pubs.rsc.org/en/content/articlelanding/2016/ta/c5ta08565a#!divAbstract